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All Printable Perovskite Solar Modules with 198 cm2 Active Area and Over 6% Efficiency

Francesca De Rossi Orcid Logo, Jenny Baker Orcid Logo, David Beynon Orcid Logo, Katherine E. A. Hooper, Simone Meroni Orcid Logo, Daniel Williams, Zhengfei Wei, Amrita Yasin, Cecile Charbonneau Orcid Logo, Eifion Jewell Orcid Logo, Trystan Watson Orcid Logo

Advanced Materials Technologies, Volume: 3, Issue: 11

Swansea University Authors: Francesca De Rossi Orcid Logo, Jenny Baker Orcid Logo, David Beynon Orcid Logo, Simone Meroni Orcid Logo, Zhengfei Wei, Cecile Charbonneau Orcid Logo, Eifion Jewell Orcid Logo, Trystan Watson Orcid Logo

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DOI (Published version): 10.1002/admt.201800156

Abstract

Perovskite solar cells based on an all printable mesoporous stack, made of overlapping titania, zirconia, and carbon layers, represent a promising device architecture for both simple, low‐cost manufacture, and outstanding stability. Here a breakthrough in the upscaling of this technology is reported...

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Published in: Advanced Materials Technologies
ISSN: 2365-709X
Published: 2018
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URI: https://cronfa.swan.ac.uk/Record/cronfa40885
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Here a breakthrough in the upscaling of this technology is reported: Screen printed modules on A4 sized conductive glass substrates, delivering power conversion efficiency (PCE) ranging from 3 to 5% at 1 sun on an unprecedented 198 cm2 active area. An increase in the PCE, due to higher VOC and fill factor, is demonstrated by patterning the TiO2 blocking layer. Furthermore, an unexpected increase of the performance is observed over time, while storing the modules in the dark, unencapsulated, at ambient conditions (with humidity increasing from 30 and 70% RH), resulting in 6.6% PCE and 6.3% stabilised at Vmax measured after over two months since fabrication. Equally impressive is the low light performance with 11 and 18% PCE achieved respectively at 200 and 1000 lux under fluorescent lighting. 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spelling 2023-02-14T15:44:39.9051862 v2 40885 2018-06-29 All Printable Perovskite Solar Modules with 198 cm2 Active Area and Over 6% Efficiency 04b56f7760ea2de5fd65985ff510d625 0000-0002-6591-5928 Francesca De Rossi Francesca De Rossi true false 6913b56f36f0c8cd34d8c9040d2df460 0000-0003-3530-1957 Jenny Baker Jenny Baker true false f5cf40043658d0b8a747ef6224019939 0000-0002-8189-9489 David Beynon David Beynon true false 78a4cf80ab2fe6cca80716b5d357d8dd 0000-0002-6901-772X Simone Meroni Simone Meroni true false e4ae52ae9b63b7b6da834c460ee3bb2d Zhengfei Wei Zhengfei Wei true false 4dc059714847cb22ed922ab058950560 0000-0001-9887-2007 Cecile Charbonneau Cecile Charbonneau true false 13dc152c178d51abfe0634445b0acf07 0000-0002-6894-2251 Eifion Jewell Eifion Jewell true false a210327b52472cfe8df9b8108d661457 0000-0002-8015-1436 Trystan Watson Trystan Watson true false 2018-06-29 EEN Perovskite solar cells based on an all printable mesoporous stack, made of overlapping titania, zirconia, and carbon layers, represent a promising device architecture for both simple, low‐cost manufacture, and outstanding stability. Here a breakthrough in the upscaling of this technology is reported: Screen printed modules on A4 sized conductive glass substrates, delivering power conversion efficiency (PCE) ranging from 3 to 5% at 1 sun on an unprecedented 198 cm2 active area. An increase in the PCE, due to higher VOC and fill factor, is demonstrated by patterning the TiO2 blocking layer. Furthermore, an unexpected increase of the performance is observed over time, while storing the modules in the dark, unencapsulated, at ambient conditions (with humidity increasing from 30 and 70% RH), resulting in 6.6% PCE and 6.3% stabilised at Vmax measured after over two months since fabrication. Equally impressive is the low light performance with 11 and 18% PCE achieved respectively at 200 and 1000 lux under fluorescent lighting. It is hoped that this demonstration of good performance on large area can unlock the viability of perovskite solar cells manufactured on an industrial scale. Journal Article Advanced Materials Technologies 3 11 2365-709X 16 11 2018 2018-11-16 10.1002/admt.201800156 COLLEGE NANME Engineering COLLEGE CODE EEN Swansea University 2023-02-14T15:44:39.9051862 2018-06-29T15:39:41.3730165 Faculty of Science and Engineering School of Engineering and Applied Sciences - Materials Science and Engineering Francesca De Rossi 0000-0002-6591-5928 1 Jenny Baker 0000-0003-3530-1957 2 David Beynon 0000-0002-8189-9489 3 Katherine E. A. Hooper 4 Simone Meroni 0000-0002-6901-772X 5 Daniel Williams 6 Zhengfei Wei 7 Amrita Yasin 8 Cecile Charbonneau 0000-0001-9887-2007 9 Eifion Jewell 0000-0002-6894-2251 10 Trystan Watson 0000-0002-8015-1436 11 0040885-16072018085224.pdf derossi2018.pdf 2018-07-16T08:52:24.1070000 Output 1018625 application/pdf Accepted Manuscript true 2019-08-13T00:00:00.0000000 true eng 0040885-16072018085251.pdf derossi-supportinginfo2018.pdf 2018-07-16T08:52:51.2370000 Output 1121016 application/pdf Supplemental material true 2019-08-13T00:00:00.0000000 true eng
title All Printable Perovskite Solar Modules with 198 cm2 Active Area and Over 6% Efficiency
spellingShingle All Printable Perovskite Solar Modules with 198 cm2 Active Area and Over 6% Efficiency
Francesca De Rossi
Jenny Baker
David Beynon
Simone Meroni
Zhengfei Wei
Cecile Charbonneau
Eifion Jewell
Trystan Watson
title_short All Printable Perovskite Solar Modules with 198 cm2 Active Area and Over 6% Efficiency
title_full All Printable Perovskite Solar Modules with 198 cm2 Active Area and Over 6% Efficiency
title_fullStr All Printable Perovskite Solar Modules with 198 cm2 Active Area and Over 6% Efficiency
title_full_unstemmed All Printable Perovskite Solar Modules with 198 cm2 Active Area and Over 6% Efficiency
title_sort All Printable Perovskite Solar Modules with 198 cm2 Active Area and Over 6% Efficiency
author_id_str_mv 04b56f7760ea2de5fd65985ff510d625
6913b56f36f0c8cd34d8c9040d2df460
f5cf40043658d0b8a747ef6224019939
78a4cf80ab2fe6cca80716b5d357d8dd
e4ae52ae9b63b7b6da834c460ee3bb2d
4dc059714847cb22ed922ab058950560
13dc152c178d51abfe0634445b0acf07
a210327b52472cfe8df9b8108d661457
author_id_fullname_str_mv 04b56f7760ea2de5fd65985ff510d625_***_Francesca De Rossi
6913b56f36f0c8cd34d8c9040d2df460_***_Jenny Baker
f5cf40043658d0b8a747ef6224019939_***_David Beynon
78a4cf80ab2fe6cca80716b5d357d8dd_***_Simone Meroni
e4ae52ae9b63b7b6da834c460ee3bb2d_***_Zhengfei Wei
4dc059714847cb22ed922ab058950560_***_Cecile Charbonneau
13dc152c178d51abfe0634445b0acf07_***_Eifion Jewell
a210327b52472cfe8df9b8108d661457_***_Trystan Watson
author Francesca De Rossi
Jenny Baker
David Beynon
Simone Meroni
Zhengfei Wei
Cecile Charbonneau
Eifion Jewell
Trystan Watson
author2 Francesca De Rossi
Jenny Baker
David Beynon
Katherine E. A. Hooper
Simone Meroni
Daniel Williams
Zhengfei Wei
Amrita Yasin
Cecile Charbonneau
Eifion Jewell
Trystan Watson
format Journal article
container_title Advanced Materials Technologies
container_volume 3
container_issue 11
publishDate 2018
institution Swansea University
issn 2365-709X
doi_str_mv 10.1002/admt.201800156
college_str Faculty of Science and Engineering
hierarchytype
hierarchy_top_id facultyofscienceandengineering
hierarchy_top_title Faculty of Science and Engineering
hierarchy_parent_id facultyofscienceandengineering
hierarchy_parent_title Faculty of Science and Engineering
department_str School of Engineering and Applied Sciences - Materials Science and Engineering{{{_:::_}}}Faculty of Science and Engineering{{{_:::_}}}School of Engineering and Applied Sciences - Materials Science and Engineering
document_store_str 1
active_str 0
description Perovskite solar cells based on an all printable mesoporous stack, made of overlapping titania, zirconia, and carbon layers, represent a promising device architecture for both simple, low‐cost manufacture, and outstanding stability. Here a breakthrough in the upscaling of this technology is reported: Screen printed modules on A4 sized conductive glass substrates, delivering power conversion efficiency (PCE) ranging from 3 to 5% at 1 sun on an unprecedented 198 cm2 active area. An increase in the PCE, due to higher VOC and fill factor, is demonstrated by patterning the TiO2 blocking layer. Furthermore, an unexpected increase of the performance is observed over time, while storing the modules in the dark, unencapsulated, at ambient conditions (with humidity increasing from 30 and 70% RH), resulting in 6.6% PCE and 6.3% stabilised at Vmax measured after over two months since fabrication. Equally impressive is the low light performance with 11 and 18% PCE achieved respectively at 200 and 1000 lux under fluorescent lighting. It is hoped that this demonstration of good performance on large area can unlock the viability of perovskite solar cells manufactured on an industrial scale.
published_date 2018-11-16T03:52:05Z
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score 11.036531

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