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High performance rigid and flexible tandem perovskite photovoltaics under mimic high-altitude platform satellite environments

Ram Datt Orcid Logo, Jinyan Guo Orcid Logo, Dong Zhou Orcid Logo, Renxing Lin Orcid Logo, Ludong Li Orcid Logo, Hairen Tan Orcid Logo, Wing Chung Tsoi Orcid Logo

Applied Physics Letters, Volume: 126, Issue: 25, Start page: 253905

Swansea University Authors: Ram Datt Orcid Logo, Wing Chung Tsoi Orcid Logo

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DOI (Published version): 10.1063/5.0272984

Abstract

Perovskite photovoltaics (PPV) have the potential to be used for aerospace applications due to, e.g., their high power-per-mass, high flexibility, and low-cost. Recent developments in narrow bandgap (NBG), wide bandgap (WBG), and tandem perovskite-based PPV devices have delivered excellent photovolt...

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Published in: Applied Physics Letters
ISSN: 0003-6951 1077-3118
Published: AIP Publishing 2025
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URI: https://cronfa.swan.ac.uk/Record/cronfa69878
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Recent developments in narrow bandgap (NBG), wide bandgap (WBG), and tandem perovskite-based PPV devices have delivered excellent photovoltaic performance for outdoor applications. In this work, we have studied NBG, WBG, and tandem (on glass and flexible substrates) PPV devices under mimic high-altitude platform satellites (HAPS) operating environment, including light irradiation (AM0), temperature (+10 to &#x2212;20 &#xB0;C), and vacuum. Furthermore, the thermal cycling (TC) (+20 to &#x2212;85 &#xB0;C) stability is also conducted for NBG, WBG, and tandem PPV devices. Tandem devices on glass and flexible substrates delivered power conversion efficiency (maximum power) of 22.98% (31.39 mW/cm2) and 21.92% (29.91 mW/cm2), respectively, under AM0 irradiation and also showed promising TC stability in the HAPS environment. Interestingly, the tandem PPV (using the NBG and WBG perovskites) retains high performance under low temperatures compared to NBG and WBG devices. 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spelling 2025-07-03T12:39:17.6307600 v2 69878 2025-07-03 High performance rigid and flexible tandem perovskite photovoltaics under mimic high-altitude platform satellite environments 350d1f64ddd9787a6eda98611dcbb8d2 0000-0003-3109-1278 Ram Datt Ram Datt true false 7e5f541df6635a9a8e1a579ff2de5d56 0000-0003-3836-5139 Wing Chung Tsoi Wing Chung Tsoi true false 2025-07-03 EAAS Perovskite photovoltaics (PPV) have the potential to be used for aerospace applications due to, e.g., their high power-per-mass, high flexibility, and low-cost. Recent developments in narrow bandgap (NBG), wide bandgap (WBG), and tandem perovskite-based PPV devices have delivered excellent photovoltaic performance for outdoor applications. In this work, we have studied NBG, WBG, and tandem (on glass and flexible substrates) PPV devices under mimic high-altitude platform satellites (HAPS) operating environment, including light irradiation (AM0), temperature (+10 to −20 °C), and vacuum. Furthermore, the thermal cycling (TC) (+20 to −85 °C) stability is also conducted for NBG, WBG, and tandem PPV devices. Tandem devices on glass and flexible substrates delivered power conversion efficiency (maximum power) of 22.98% (31.39 mW/cm2) and 21.92% (29.91 mW/cm2), respectively, under AM0 irradiation and also showed promising TC stability in the HAPS environment. Interestingly, the tandem PPV (using the NBG and WBG perovskites) retains high performance under low temperatures compared to NBG and WBG devices. Therefore, it demonstrated the promising potential of Tandem PPV for HAPS application. Journal Article Applied Physics Letters 126 25 253905 AIP Publishing 0003-6951 1077-3118 24 6 2025 2025-06-24 10.1063/5.0272984 COLLEGE NANME Engineering and Applied Sciences School COLLEGE CODE EAAS Swansea University SU Library paid the OA fee (TA Institutional Deal) Engineering and Physical Sciences Research Council Grant: EP/T028513/1; National Natural Science Foundation of China Grants: U21A2076, 62305150, 52427803, and 62474086; Natural Science Foundation of Jiangsu Province Grants: BK20232022, BE2022021, and BE2022026. 2025-07-03T12:39:17.6307600 2025-07-03T12:27:23.5652963 Faculty of Science and Engineering School of Engineering and Applied Sciences - Materials Science and Engineering Ram Datt 0000-0003-3109-1278 1 Jinyan Guo 0009-0003-8892-2738 2 Dong Zhou 0009-0006-5704-1585 3 Renxing Lin 0000-0001-5710-7181 4 Ludong Li 0000-0002-7023-1985 5 Hairen Tan 0000-0003-0821-476X 6 Wing Chung Tsoi 0000-0003-3836-5139 7 69878__34656__2b276a7e82324b3e8d13fb4d091dc30a.pdf 69878.VOR.pdf 2025-07-03T12:32:56.9331750 Output 2507047 application/pdf Version of Record true © 2025 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license true eng https://creativecommons.org/licenses/by/4.0/
title High performance rigid and flexible tandem perovskite photovoltaics under mimic high-altitude platform satellite environments
spellingShingle High performance rigid and flexible tandem perovskite photovoltaics under mimic high-altitude platform satellite environments
Ram Datt
Wing Chung Tsoi
title_short High performance rigid and flexible tandem perovskite photovoltaics under mimic high-altitude platform satellite environments
title_full High performance rigid and flexible tandem perovskite photovoltaics under mimic high-altitude platform satellite environments
title_fullStr High performance rigid and flexible tandem perovskite photovoltaics under mimic high-altitude platform satellite environments
title_full_unstemmed High performance rigid and flexible tandem perovskite photovoltaics under mimic high-altitude platform satellite environments
title_sort High performance rigid and flexible tandem perovskite photovoltaics under mimic high-altitude platform satellite environments
author_id_str_mv 350d1f64ddd9787a6eda98611dcbb8d2
7e5f541df6635a9a8e1a579ff2de5d56
author_id_fullname_str_mv 350d1f64ddd9787a6eda98611dcbb8d2_***_Ram Datt
7e5f541df6635a9a8e1a579ff2de5d56_***_Wing Chung Tsoi
author Ram Datt
Wing Chung Tsoi
author2 Ram Datt
Jinyan Guo
Dong Zhou
Renxing Lin
Ludong Li
Hairen Tan
Wing Chung Tsoi
format Journal article
container_title Applied Physics Letters
container_volume 126
container_issue 25
container_start_page 253905
publishDate 2025
institution Swansea University
issn 0003-6951
1077-3118
doi_str_mv 10.1063/5.0272984
publisher AIP Publishing
college_str Faculty of Science and Engineering
hierarchytype
hierarchy_top_id facultyofscienceandengineering
hierarchy_top_title Faculty of Science and Engineering
hierarchy_parent_id facultyofscienceandengineering
hierarchy_parent_title Faculty of Science and Engineering
department_str School of Engineering and Applied Sciences - Materials Science and Engineering{{{_:::_}}}Faculty of Science and Engineering{{{_:::_}}}School of Engineering and Applied Sciences - Materials Science and Engineering
document_store_str 1
active_str 0
description Perovskite photovoltaics (PPV) have the potential to be used for aerospace applications due to, e.g., their high power-per-mass, high flexibility, and low-cost. Recent developments in narrow bandgap (NBG), wide bandgap (WBG), and tandem perovskite-based PPV devices have delivered excellent photovoltaic performance for outdoor applications. In this work, we have studied NBG, WBG, and tandem (on glass and flexible substrates) PPV devices under mimic high-altitude platform satellites (HAPS) operating environment, including light irradiation (AM0), temperature (+10 to −20 °C), and vacuum. Furthermore, the thermal cycling (TC) (+20 to −85 °C) stability is also conducted for NBG, WBG, and tandem PPV devices. Tandem devices on glass and flexible substrates delivered power conversion efficiency (maximum power) of 22.98% (31.39 mW/cm2) and 21.92% (29.91 mW/cm2), respectively, under AM0 irradiation and also showed promising TC stability in the HAPS environment. Interestingly, the tandem PPV (using the NBG and WBG perovskites) retains high performance under low temperatures compared to NBG and WBG devices. Therefore, it demonstrated the promising potential of Tandem PPV for HAPS application.
published_date 2025-06-24T12:33:14Z
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score 11.08895

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