No Cover Image

Journal article 364 views 117 downloads

Quantum dots solar cells under mimic high altitude platform satellites environments

Ram Datt Orcid Logo, Xin Wen Orcid Logo, Xiaobo Ding Orcid Logo, Zeke Liu Orcid Logo, Wanli Ma Orcid Logo, Wing Chung Tsoi Orcid Logo

Applied Physics Letters, Volume: 126, Issue: 25, Start page: 253904

Swansea University Authors: Ram Datt Orcid Logo, Wing Chung Tsoi Orcid Logo

  • 69874.VOR.pdf

    PDF | Version of Record

    C 2025 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license.

    Download (3.19MB)

Check full text

DOI (Published version): 10.1063/5.0278791

Abstract

Quantum dot solar cells are solution-processable, lightweight, and low-cost, and their long-term stability makes them attractive to explore for aerospace applications. In this work, we have studied lead sulfide (PbS) colloidal quantum dot solar cells (CQDSCs) using three different types of hole tran...

Full description

Published in: Applied Physics Letters
ISSN: 0003-6951 1077-3118
Published: AIP Publishing 2025
Online Access: Check full text

URI: https://cronfa.swan.ac.uk/Record/cronfa69874
Abstract: Quantum dot solar cells are solution-processable, lightweight, and low-cost, and their long-term stability makes them attractive to explore for aerospace applications. In this work, we have studied lead sulfide (PbS) colloidal quantum dot solar cells (CQDSCs) using three different types of hole transport layer combinations, such as PbS-MPA/PbS-MPA (PbS-MPA), P3HT/PTAA (P3HT), and PBDB-T/MoO3(PBDB-T), under mimic working environmental conditions for high altitude platform satellites (HAPS). It includes ultraviolet rich solar irradiation (AM0), low temperature conditions (+10 to −20 °C), and low pressure. The thermal cycling (considering change in temperature at day–night) measurements were also conducted. The device performance under a broad range of temperatures from +80 to −100 °C was also included. The devices delivered power conversion efficiency (PCE) of 9.46 (8.41), 9.68 (7.86), and 11.77 (10.75)% for PbS-MPA, P3HT, and PBDB-T devices under AM1.5G(AM0), respectively. PbS-MPA devices maintain the PCE and slightly improve their performance under low temperatures (from 0 down to −100 °C). Meanwhile, the P3HT and PBDB-T-based CQDSCs devices started to decline in PCE significantly from −40 and +10 °C, respectively. Furthermore, PbS-MPA devices show excellent thermal cycling stability, making them attractive for further exploration for aerospace applications.
College: Faculty of Science and Engineering
Funders: Engineering and Physical Sciences Research Council Grant: EP/T028513/1; National Natural Science Foundation of China Grant: 52372215
Issue: 25
Start Page: 253904