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High performance rigid and flexible tandem perovskite photovoltaics under mimic high-altitude platform satellite environments

Ram Datt Orcid Logo, Jinyan Guo Orcid Logo, Dong Zhou Orcid Logo, Renxing Lin Orcid Logo, Ludong Li Orcid Logo, Hairen Tan Orcid Logo, Wing Chung Tsoi Orcid Logo

Applied Physics Letters, Volume: 126, Issue: 25, Start page: 253905

Swansea University Authors: Ram Datt Orcid Logo, Wing Chung Tsoi Orcid Logo

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DOI (Published version): 10.1063/5.0272984

Abstract

Perovskite photovoltaics (PPV) have the potential to be used for aerospace applications due to, e.g., their high power-per-mass, high flexibility, and low-cost. Recent developments in narrow bandgap (NBG), wide bandgap (WBG), and tandem perovskite-based PPV devices have delivered excellent photovolt...

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Published in: Applied Physics Letters
ISSN: 0003-6951 1077-3118
Published: AIP Publishing 2025
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URI: https://cronfa.swan.ac.uk/Record/cronfa69878
Abstract: Perovskite photovoltaics (PPV) have the potential to be used for aerospace applications due to, e.g., their high power-per-mass, high flexibility, and low-cost. Recent developments in narrow bandgap (NBG), wide bandgap (WBG), and tandem perovskite-based PPV devices have delivered excellent photovoltaic performance for outdoor applications. In this work, we have studied NBG, WBG, and tandem (on glass and flexible substrates) PPV devices under mimic high-altitude platform satellites (HAPS) operating environment, including light irradiation (AM0), temperature (+10 to −20 °C), and vacuum. Furthermore, the thermal cycling (TC) (+20 to −85 °C) stability is also conducted for NBG, WBG, and tandem PPV devices. Tandem devices on glass and flexible substrates delivered power conversion efficiency (maximum power) of 22.98% (31.39 mW/cm2) and 21.92% (29.91 mW/cm2), respectively, under AM0 irradiation and also showed promising TC stability in the HAPS environment. Interestingly, the tandem PPV (using the NBG and WBG perovskites) retains high performance under low temperatures compared to NBG and WBG devices. Therefore, it demonstrated the promising potential of Tandem PPV for HAPS application.
College: Faculty of Science and Engineering
Funders: Engineering and Physical Sciences Research Council Grant: EP/T028513/1; National Natural Science Foundation of China Grants: U21A2076, 62305150, 52427803, and 62474086; Natural Science Foundation of Jiangsu Province Grants: BK20232022, BE2022021, and BE2022026.
Issue: 25
Start Page: 253905