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Process‐Structure‐Formulation Interactions for Enhanced Sodium Ion Battery Development: A Review

Anne Sawhney Orcid Logo, Malik Wahid, Santanu Mukherjee, Rebecca Griffin, Alexander Roberts, Satishchandra Ogale, Jenny Baker

ChemPhysChem, Volume: 23, Issue: 5

Swansea University Authors: Anne Sawhney Orcid Logo, Santanu Mukherjee, Jenny Baker

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DOI (Published version): 10.1002/cphc.202100860

Abstract

Before the viability of a cell formulation can be assessed for implementation in commercial sodium ion batteries, processes applied in cell production should be validated and optimized. This review summarizes the steps performed in constructing sodium ion (Na-ion) cells at research scale, highlighti...

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Published in: ChemPhysChem
ISSN: 1439-4235 1439-7641
Published: Wiley 2022
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URI: https://cronfa.swan.ac.uk/Record/cronfa59151
first_indexed 2022-01-11T16:54:45Z
last_indexed 2023-01-11T14:40:13Z
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spelling 2022-08-17T14:50:40.7807410 v2 59151 2022-01-11 Process‐Structure‐Formulation Interactions for Enhanced Sodium Ion Battery Development: A Review 17a538477108587c0abd065ee891f3a3 0000-0003-3242-6789 Anne Sawhney Anne Sawhney true false 34081bd5f2ebaa184716285d94d62828 Santanu Mukherjee Santanu Mukherjee true false 6913b56f36f0c8cd34d8c9040d2df460 Jenny Baker Jenny Baker true false 2022-01-11 EAAS Before the viability of a cell formulation can be assessed for implementation in commercial sodium ion batteries, processes applied in cell production should be validated and optimized. This review summarizes the steps performed in constructing sodium ion (Na-ion) cells at research scale, highlighting parameters and techniques that are likely to impact measured cycling performance. Consistent process-structure-performance links have been established for typical lithium-ion (Li-ion) cells, which can guide hypotheses to test in Na-ion cells. Liquid electrolyte viscosity, sequence of mixing electrode slurries, rate of drying electrodes and cycling characteristics of formation were found critical to the reported capacity of laboratory cells. Based on the observed importance of processing to battery performance outcomes, the current focus on novel materials in Na-ion research should be balanced with deeper investigation into mechanistic changes of cell components during and after production, to better inform future designs of these promising batteries. Journal Article ChemPhysChem 23 5 Wiley 1439-4235 1439-7641 cell processing; electrochemistry; electrolyte casting; Na-ion; slurry mixing 4 3 2022 2022-03-04 10.1002/cphc.202100860 COLLEGE NANME Engineering and Applied Sciences School COLLEGE CODE EAAS Swansea University SU Library paid the OA fee (TA Institutional Deal) Engineering and Physical Sciences Research Council (EPSRC); Materials Research Hub for Energy Conversion, Capture, and Storage (M-RHEX). Grant Number: EP/R023581/1; ECR Fellowship NoRESt. Grant Number: EP/S03711X/1; SPECIFIC Innovation and Knowledge Centre. Grant Numbers: EP/N020863/1, EP/P030831/1; UKRI Global Challenge Research Fund project, SUNRISE. Grant Number: EP/P032591/1; Department of Science and Technology (DST) India Grant. Grant Number: DST/INSPIRE/04/2017/002798; European Social Fund via the Welsh Government. Grant Number: c80816; Engineering and Physical Sciences Research Council. Grant Number: EP/S02252X/1 2022-08-17T14:50:40.7807410 2022-01-11T16:53:17.1935356 Faculty of Science and Engineering School of Aerospace, Civil, Electrical, General and Mechanical Engineering - Mechanical Engineering Anne Sawhney 0000-0003-3242-6789 1 Malik Wahid 2 Santanu Mukherjee 3 Rebecca Griffin 4 Alexander Roberts 5 Satishchandra Ogale 6 Jenny Baker 7 59151__22518__f99f72b31a33457daf1e91c59fd7ce6d.pdf 59151.pdf 2022-03-04T14:27:27.2257267 Output 2728758 application/pdf Version of Record true © 2022 The Authors. This is an open access article under the terms of the Creative Commons Attribution License true eng http://creativecommons.org/licenses/by/4.0/
title Process‐Structure‐Formulation Interactions for Enhanced Sodium Ion Battery Development: A Review
spellingShingle Process‐Structure‐Formulation Interactions for Enhanced Sodium Ion Battery Development: A Review
Anne Sawhney
Santanu Mukherjee
Jenny Baker
title_short Process‐Structure‐Formulation Interactions for Enhanced Sodium Ion Battery Development: A Review
title_full Process‐Structure‐Formulation Interactions for Enhanced Sodium Ion Battery Development: A Review
title_fullStr Process‐Structure‐Formulation Interactions for Enhanced Sodium Ion Battery Development: A Review
title_full_unstemmed Process‐Structure‐Formulation Interactions for Enhanced Sodium Ion Battery Development: A Review
title_sort Process‐Structure‐Formulation Interactions for Enhanced Sodium Ion Battery Development: A Review
author_id_str_mv 17a538477108587c0abd065ee891f3a3
34081bd5f2ebaa184716285d94d62828
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author_id_fullname_str_mv 17a538477108587c0abd065ee891f3a3_***_Anne Sawhney
34081bd5f2ebaa184716285d94d62828_***_Santanu Mukherjee
6913b56f36f0c8cd34d8c9040d2df460_***_Jenny Baker
author Anne Sawhney
Santanu Mukherjee
Jenny Baker
author2 Anne Sawhney
Malik Wahid
Santanu Mukherjee
Rebecca Griffin
Alexander Roberts
Satishchandra Ogale
Jenny Baker
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container_title ChemPhysChem
container_volume 23
container_issue 5
publishDate 2022
institution Swansea University
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doi_str_mv 10.1002/cphc.202100860
publisher Wiley
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department_str School of Aerospace, Civil, Electrical, General and Mechanical Engineering - Mechanical Engineering{{{_:::_}}}Faculty of Science and Engineering{{{_:::_}}}School of Aerospace, Civil, Electrical, General and Mechanical Engineering - Mechanical Engineering
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description Before the viability of a cell formulation can be assessed for implementation in commercial sodium ion batteries, processes applied in cell production should be validated and optimized. This review summarizes the steps performed in constructing sodium ion (Na-ion) cells at research scale, highlighting parameters and techniques that are likely to impact measured cycling performance. Consistent process-structure-performance links have been established for typical lithium-ion (Li-ion) cells, which can guide hypotheses to test in Na-ion cells. Liquid electrolyte viscosity, sequence of mixing electrode slurries, rate of drying electrodes and cycling characteristics of formation were found critical to the reported capacity of laboratory cells. Based on the observed importance of processing to battery performance outcomes, the current focus on novel materials in Na-ion research should be balanced with deeper investigation into mechanistic changes of cell components during and after production, to better inform future designs of these promising batteries.
published_date 2022-03-04T02:25:23Z
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