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Homogeneous and highly controlled deposition of low viscosity inks and application on fully printable perovskite solar cells

Simone Meroni Orcid Logo, Youmna Mouhamad, Francesca De Rossi Orcid Logo, Adam Pockett, Jenny Baker Orcid Logo, Renán Escalante, Justin Searle Orcid Logo, Matt Carnie Orcid Logo, Eifion Jewell Orcid Logo, Gerko Oskam, Trystan Watson Orcid Logo

Science and Technology of Advanced Materials, Volume: 19, Issue: 1, Pages: 1 - 9

Swansea University Authors: Simone Meroni Orcid Logo, Youmna Mouhamad, Francesca De Rossi Orcid Logo, Adam Pockett, Jenny Baker Orcid Logo, Justin Searle Orcid Logo, Matt Carnie Orcid Logo, Eifion Jewell Orcid Logo, Trystan Watson Orcid Logo

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DOI (Published version): 10.1080/14686996.2017.1406777

Abstract

The fully printed, hole-transporter-free carbon perovskite solar cell structure incorporating a triple mesoscopic layer has emerged as a possible frontrunner for early industrialisation. It is an attractive structure because it can be fabricated by the simple sequential screen printing and sintering...

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Published in: Science and Technology of Advanced Materials
ISSN: 1468-6996 1878-5514
Published: Taylor & Francis 2018
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URI: https://cronfa.swan.ac.uk/Record/cronfa37650
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It is an attractive structure because it can be fabricated by the simple sequential screen printing and sintering of titania, zirconia, and carbon. The device is finalised by manual dropping of a perovskite precursor solution onto the carbon which subsequently infiltrates. This stage in device fabrication is inhomogeneous, ineffective for large areas, and prone to human error. Here we introduce an automated deposition and infiltration system using a robotic dispenser and mesh which delivers the perovskite precursor uniformly to the carbon surface over a large area. It has been successfully used to prepare perovskite solar cells with over 9% efficiency. Cells, prepared by this robotic mesh deposition, showed comparable performance to reference cells, made by standard drop deposition, confirming this approach to be effective and reliable. 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spelling 2020-06-30T11:42:08.7062311 v2 37650 2017-12-18 Homogeneous and highly controlled deposition of low viscosity inks and application on fully printable perovskite solar cells 78a4cf80ab2fe6cca80716b5d357d8dd 0000-0002-6901-772X Simone Meroni Simone Meroni true false 24a6a0a4d08557112dfcfbcdb07d7013 Youmna Mouhamad Youmna Mouhamad true false 04b56f7760ea2de5fd65985ff510d625 0000-0002-6591-5928 Francesca De Rossi Francesca De Rossi true false de06433fccc0514dcf45aa9d1fc5c60f Adam Pockett Adam Pockett true false 6913b56f36f0c8cd34d8c9040d2df460 0000-0003-3530-1957 Jenny Baker Jenny Baker true false 0e3f2c3812f181eaed11c45554d4cdd0 0000-0003-1101-075X Justin Searle Justin Searle true false 73b367694366a646b90bb15db32bb8c0 0000-0002-4232-1967 Matt Carnie Matt Carnie true false 13dc152c178d51abfe0634445b0acf07 0000-0002-6894-2251 Eifion Jewell Eifion Jewell true false a210327b52472cfe8df9b8108d661457 0000-0002-8015-1436 Trystan Watson Trystan Watson true false 2017-12-18 MTLS The fully printed, hole-transporter-free carbon perovskite solar cell structure incorporating a triple mesoscopic layer has emerged as a possible frontrunner for early industrialisation. It is an attractive structure because it can be fabricated by the simple sequential screen printing and sintering of titania, zirconia, and carbon. The device is finalised by manual dropping of a perovskite precursor solution onto the carbon which subsequently infiltrates. This stage in device fabrication is inhomogeneous, ineffective for large areas, and prone to human error. Here we introduce an automated deposition and infiltration system using a robotic dispenser and mesh which delivers the perovskite precursor uniformly to the carbon surface over a large area. It has been successfully used to prepare perovskite solar cells with over 9% efficiency. Cells, prepared by this robotic mesh deposition, showed comparable performance to reference cells, made by standard drop deposition, confirming this approach to be effective and reliable. X-ray diffraction and Raman spectroscopy were used to confirm the uniformity of the deposition over a large area. Journal Article Science and Technology of Advanced Materials 19 1 1 9 Taylor & Francis 1468-6996 1878-5514 Solar cell, up-scaling, carbon, perovskite, printing, Raman, mapping 31 12 2018 2018-12-31 10.1080/14686996.2017.1406777 https://www.tandfonline.com/doi/full/10.1080/14686996.2017.1406777 COLLEGE NANME Materials Science and Engineering COLLEGE CODE MTLS Swansea University 2020-06-30T11:42:08.7062311 2017-12-18T20:45:26.2722658 Faculty of Science and Engineering School of Aerospace, Civil, Electrical, General and Mechanical Engineering - Mechanical Engineering Simone Meroni 0000-0002-6901-772X 1 Youmna Mouhamad 2 Francesca De Rossi 0000-0002-6591-5928 3 Adam Pockett 4 Jenny Baker 0000-0003-3530-1957 5 Renán Escalante 6 Justin Searle 0000-0003-1101-075X 7 Matt Carnie 0000-0002-4232-1967 8 Eifion Jewell 0000-0002-6894-2251 9 Gerko Oskam 10 Trystan Watson 0000-0002-8015-1436 11 0037650-02012018152407.pdf meroni2017.pdf 2018-01-02T15:24:07.5470000 Output 1204985 application/pdf Version of Record true 2018-01-02T00:00:00.0000000 true eng
title Homogeneous and highly controlled deposition of low viscosity inks and application on fully printable perovskite solar cells
spellingShingle Homogeneous and highly controlled deposition of low viscosity inks and application on fully printable perovskite solar cells
Simone Meroni
Youmna Mouhamad
Francesca De Rossi
Adam Pockett
Jenny Baker
Justin Searle
Matt Carnie
Eifion Jewell
Trystan Watson
title_short Homogeneous and highly controlled deposition of low viscosity inks and application on fully printable perovskite solar cells
title_full Homogeneous and highly controlled deposition of low viscosity inks and application on fully printable perovskite solar cells
title_fullStr Homogeneous and highly controlled deposition of low viscosity inks and application on fully printable perovskite solar cells
title_full_unstemmed Homogeneous and highly controlled deposition of low viscosity inks and application on fully printable perovskite solar cells
title_sort Homogeneous and highly controlled deposition of low viscosity inks and application on fully printable perovskite solar cells
author_id_str_mv 78a4cf80ab2fe6cca80716b5d357d8dd
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author_id_fullname_str_mv 78a4cf80ab2fe6cca80716b5d357d8dd_***_Simone Meroni
24a6a0a4d08557112dfcfbcdb07d7013_***_Youmna Mouhamad
04b56f7760ea2de5fd65985ff510d625_***_Francesca De Rossi
de06433fccc0514dcf45aa9d1fc5c60f_***_Adam Pockett
6913b56f36f0c8cd34d8c9040d2df460_***_Jenny Baker
0e3f2c3812f181eaed11c45554d4cdd0_***_Justin Searle
73b367694366a646b90bb15db32bb8c0_***_Matt Carnie
13dc152c178d51abfe0634445b0acf07_***_Eifion Jewell
a210327b52472cfe8df9b8108d661457_***_Trystan Watson
author Simone Meroni
Youmna Mouhamad
Francesca De Rossi
Adam Pockett
Jenny Baker
Justin Searle
Matt Carnie
Eifion Jewell
Trystan Watson
author2 Simone Meroni
Youmna Mouhamad
Francesca De Rossi
Adam Pockett
Jenny Baker
Renán Escalante
Justin Searle
Matt Carnie
Eifion Jewell
Gerko Oskam
Trystan Watson
format Journal article
container_title Science and Technology of Advanced Materials
container_volume 19
container_issue 1
container_start_page 1
publishDate 2018
institution Swansea University
issn 1468-6996
1878-5514
doi_str_mv 10.1080/14686996.2017.1406777
publisher Taylor & Francis
college_str Faculty of Science and Engineering
hierarchytype
hierarchy_top_id facultyofscienceandengineering
hierarchy_top_title Faculty of Science and Engineering
hierarchy_parent_id facultyofscienceandengineering
hierarchy_parent_title Faculty of Science and Engineering
department_str School of Aerospace, Civil, Electrical, General and Mechanical Engineering - Mechanical Engineering{{{_:::_}}}Faculty of Science and Engineering{{{_:::_}}}School of Aerospace, Civil, Electrical, General and Mechanical Engineering - Mechanical Engineering
url https://www.tandfonline.com/doi/full/10.1080/14686996.2017.1406777
document_store_str 1
active_str 0
description The fully printed, hole-transporter-free carbon perovskite solar cell structure incorporating a triple mesoscopic layer has emerged as a possible frontrunner for early industrialisation. It is an attractive structure because it can be fabricated by the simple sequential screen printing and sintering of titania, zirconia, and carbon. The device is finalised by manual dropping of a perovskite precursor solution onto the carbon which subsequently infiltrates. This stage in device fabrication is inhomogeneous, ineffective for large areas, and prone to human error. Here we introduce an automated deposition and infiltration system using a robotic dispenser and mesh which delivers the perovskite precursor uniformly to the carbon surface over a large area. It has been successfully used to prepare perovskite solar cells with over 9% efficiency. Cells, prepared by this robotic mesh deposition, showed comparable performance to reference cells, made by standard drop deposition, confirming this approach to be effective and reliable. X-ray diffraction and Raman spectroscopy were used to confirm the uniformity of the deposition over a large area.
published_date 2018-12-31T03:47:27Z
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score 11.013395

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