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High throughput fabrication of mesoporous carbon perovskite solar cells

Jenny Baker Orcid Logo, Katherine Hooper, Simone Meroni Orcid Logo, Adam Pockett, James McGettrick Orcid Logo, Zhengfei Wei, Renán Escalante, Gerko Oskam, Matt Carnie Orcid Logo, Trystan Watson Orcid Logo

Journal of Materials Chemistry A, Volume: 5, Issue: 35, Pages: 18643 - 18650

Swansea University Authors: Jenny Baker Orcid Logo, Katherine Hooper, Simone Meroni Orcid Logo, Adam Pockett, James McGettrick Orcid Logo, Zhengfei Wei, Matt Carnie Orcid Logo, Trystan Watson Orcid Logo

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DOI (Published version): 10.1039/C7TA05674E

Abstract

The screen printed mesoporous carbon perovskite solar cell has great potential for commercialisation due to its scalable deposition processes and use of inexpensive materials. However, each layer requires long high temperature heating steps to achieve the necessary sintering and porosity, which is v...

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Published in: Journal of Materials Chemistry A
ISSN: 2050-7488 2050-7496
Published: 2017
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URI: https://cronfa.swan.ac.uk/Record/cronfa34942
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However, each layer requires long high temperature heating steps to achieve the necessary sintering and porosity, which is very time and energy intensive for large scale production. Near infrared processing is demonstrated here to reduce the heating time of mesoporous layers within a fully printed lead halide perovskite solar cell from 2 hours to 30 seconds. A stabilised efficiency of 11% was achieved by processing in 30 seconds, identical to that of devices heated in 2 hours. For the first time the effect of residual binder in the carbon electrode on the electron lifetime and charge transfer within devices has been investigated. 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spelling 2020-12-15T10:10:57.8782512 v2 34942 2017-08-21 High throughput fabrication of mesoporous carbon perovskite solar cells 6913b56f36f0c8cd34d8c9040d2df460 0000-0003-3530-1957 Jenny Baker Jenny Baker true false 3607f6787dc810c0ed1fdc49ea2b5e63 Katherine Hooper Katherine Hooper true false 78a4cf80ab2fe6cca80716b5d357d8dd 0000-0002-6901-772X Simone Meroni Simone Meroni true false de06433fccc0514dcf45aa9d1fc5c60f Adam Pockett Adam Pockett true false bdbacc591e2de05180e0fd3cc13fa480 0000-0002-7719-2958 James McGettrick James McGettrick true false e4ae52ae9b63b7b6da834c460ee3bb2d Zhengfei Wei Zhengfei Wei true false 73b367694366a646b90bb15db32bb8c0 0000-0002-4232-1967 Matt Carnie Matt Carnie true false a210327b52472cfe8df9b8108d661457 0000-0002-8015-1436 Trystan Watson Trystan Watson true false 2017-08-21 MECH The screen printed mesoporous carbon perovskite solar cell has great potential for commercialisation due to its scalable deposition processes and use of inexpensive materials. However, each layer requires long high temperature heating steps to achieve the necessary sintering and porosity, which is very time and energy intensive for large scale production. Near infrared processing is demonstrated here to reduce the heating time of mesoporous layers within a fully printed lead halide perovskite solar cell from 2 hours to 30 seconds. A stabilised efficiency of 11% was achieved by processing in 30 seconds, identical to that of devices heated in 2 hours. For the first time the effect of residual binder in the carbon electrode on the electron lifetime and charge transfer within devices has been investigated. Furthermore cross section EDX mapping of perovskite infiltration provides a greater understanding into the processing requirements of these devices vital to enable commercialisation. Journal Article Journal of Materials Chemistry A 5 35 18643 18650 2050-7488 2050-7496 21 9 2017 2017-09-21 10.1039/C7TA05674E COLLEGE NANME Mechanical Engineering COLLEGE CODE MECH Swansea University 2020-12-15T10:10:57.8782512 2017-08-21T12:07:08.2747632 Faculty of Science and Engineering School of Engineering and Applied Sciences - Materials Science and Engineering Jenny Baker 0000-0003-3530-1957 1 Katherine Hooper 2 Simone Meroni 0000-0002-6901-772X 3 Adam Pockett 4 James McGettrick 0000-0002-7719-2958 5 Zhengfei Wei 6 Renán Escalante 7 Gerko Oskam 8 Matt Carnie 0000-0002-4232-1967 9 Trystan Watson 0000-0002-8015-1436 10 0034942-04102017110736.pdf baker2017.pdf 2017-10-04T11:07:36.5730000 Output 884696 application/pdf Accepted Manuscript true 2018-08-08T00:00:00.0000000 true eng
title High throughput fabrication of mesoporous carbon perovskite solar cells
spellingShingle High throughput fabrication of mesoporous carbon perovskite solar cells
Jenny Baker
Katherine Hooper
Simone Meroni
Adam Pockett
James McGettrick
Zhengfei Wei
Matt Carnie
Trystan Watson
title_short High throughput fabrication of mesoporous carbon perovskite solar cells
title_full High throughput fabrication of mesoporous carbon perovskite solar cells
title_fullStr High throughput fabrication of mesoporous carbon perovskite solar cells
title_full_unstemmed High throughput fabrication of mesoporous carbon perovskite solar cells
title_sort High throughput fabrication of mesoporous carbon perovskite solar cells
author_id_str_mv 6913b56f36f0c8cd34d8c9040d2df460
3607f6787dc810c0ed1fdc49ea2b5e63
78a4cf80ab2fe6cca80716b5d357d8dd
de06433fccc0514dcf45aa9d1fc5c60f
bdbacc591e2de05180e0fd3cc13fa480
e4ae52ae9b63b7b6da834c460ee3bb2d
73b367694366a646b90bb15db32bb8c0
a210327b52472cfe8df9b8108d661457
author_id_fullname_str_mv 6913b56f36f0c8cd34d8c9040d2df460_***_Jenny Baker
3607f6787dc810c0ed1fdc49ea2b5e63_***_Katherine Hooper
78a4cf80ab2fe6cca80716b5d357d8dd_***_Simone Meroni
de06433fccc0514dcf45aa9d1fc5c60f_***_Adam Pockett
bdbacc591e2de05180e0fd3cc13fa480_***_James McGettrick
e4ae52ae9b63b7b6da834c460ee3bb2d_***_Zhengfei Wei
73b367694366a646b90bb15db32bb8c0_***_Matt Carnie
a210327b52472cfe8df9b8108d661457_***_Trystan Watson
author Jenny Baker
Katherine Hooper
Simone Meroni
Adam Pockett
James McGettrick
Zhengfei Wei
Matt Carnie
Trystan Watson
author2 Jenny Baker
Katherine Hooper
Simone Meroni
Adam Pockett
James McGettrick
Zhengfei Wei
Renán Escalante
Gerko Oskam
Matt Carnie
Trystan Watson
format Journal article
container_title Journal of Materials Chemistry A
container_volume 5
container_issue 35
container_start_page 18643
publishDate 2017
institution Swansea University
issn 2050-7488
2050-7496
doi_str_mv 10.1039/C7TA05674E
college_str Faculty of Science and Engineering
hierarchytype
hierarchy_top_id facultyofscienceandengineering
hierarchy_top_title Faculty of Science and Engineering
hierarchy_parent_id facultyofscienceandengineering
hierarchy_parent_title Faculty of Science and Engineering
department_str School of Engineering and Applied Sciences - Materials Science and Engineering{{{_:::_}}}Faculty of Science and Engineering{{{_:::_}}}School of Engineering and Applied Sciences - Materials Science and Engineering
document_store_str 1
active_str 0
description The screen printed mesoporous carbon perovskite solar cell has great potential for commercialisation due to its scalable deposition processes and use of inexpensive materials. However, each layer requires long high temperature heating steps to achieve the necessary sintering and porosity, which is very time and energy intensive for large scale production. Near infrared processing is demonstrated here to reduce the heating time of mesoporous layers within a fully printed lead halide perovskite solar cell from 2 hours to 30 seconds. A stabilised efficiency of 11% was achieved by processing in 30 seconds, identical to that of devices heated in 2 hours. For the first time the effect of residual binder in the carbon electrode on the electron lifetime and charge transfer within devices has been investigated. Furthermore cross section EDX mapping of perovskite infiltration provides a greater understanding into the processing requirements of these devices vital to enable commercialisation.
published_date 2017-09-21T03:43:23Z
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score 11.036334

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