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Development of polysulfone-nanohybrid membranes using ZnO-GO composite for enhanced antifouling and antibacterial control

Ying Tao Chung, Ebrahim Mahmoudi, Abdul Wahab Mohammad, Abdelbaki Benamor, Daniel Johnson Orcid Logo, Nidal Hilal

Desalination, Volume: 402, Pages: 123 - 132

Swansea University Authors: Daniel Johnson Orcid Logo, Nidal Hilal

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DOI (Published version): 10.1016/j.desal.2016.09.030

Abstract

Zinc oxide nanoparticles were well-known for the enhanced antifouling and antibacterial properties which could be beneficial for membrane processes in desalination. The functionalization of ZnO onto graphene oxide nanoplates was targeted for better distribution. Both ZnO and ZnO-GO NPs were synthesi...

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Published in: Desalination
ISSN: 0011-9164
Published: 2017
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URI: https://cronfa.swan.ac.uk/Record/cronfa30211
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first_indexed 2016-10-11T18:27:10Z
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spelling 2016-10-12T08:59:29.2566200 v2 30211 2016-09-26 Development of polysulfone-nanohybrid membranes using ZnO-GO composite for enhanced antifouling and antibacterial control 4bdcc306062428d2715b0dd308cc092f 0000-0001-6921-0389 Daniel Johnson Daniel Johnson true false 3acba771241d878c8e35ff464aec0342 Nidal Hilal Nidal Hilal true false 2016-09-26 Zinc oxide nanoparticles were well-known for the enhanced antifouling and antibacterial properties which could be beneficial for membrane processes in desalination. The functionalization of ZnO onto graphene oxide nanoplates was targeted for better distribution. Both ZnO and ZnO-GO NPs were synthesized using sol-gel method. The nanoparticles characteristics were checked with XRD, TEM, and FESEM. The nanohybrid membranes were fabricated via wet phase inversion technique and embedded with various percentage of ZnO (1, 2, 3 wt%) and ZnO-GO (0.1, 0.3, 0.6 wt%) nanoparticles. All the membranes with nanoparticles incorporation exhibited improved membrane properties in comparison with the pristine PSF membrane. The best membrane performance was shown in membrane with 2 wt% of ZnO and 0.6 wt% of ZnO-GO. These two membranes presented significantly improved performance such as enhanced hydrophilicity, high permeability and porosity, improved humic acid rejection rate as well as good antifouling and antibacterial control. To an extent, the excellent antimicrobial ability of these nanohybrid membranes appeared as appropriate candidate to contribute or overcome bio-fouling issues in applications such as brackish water or seawater desalination. Hence, ZnO and ZnO-GO NPs were superb nanomaterials in the fabrication of PSF-nanohybrid membranes. The use of GO nanoplates allowed reduction of ZnO composition by up to 5 times while showing similar performances. Journal Article Desalination 402 123 132 0011-9164 16 1 2017 2017-01-16 10.1016/j.desal.2016.09.030 COLLEGE NANME COLLEGE CODE Swansea University 2016-10-12T08:59:29.2566200 2016-09-26T10:00:53.6573369 Faculty of Science and Engineering School of Engineering and Applied Sciences - Uncategorised Ying Tao Chung 1 Ebrahim Mahmoudi 2 Abdul Wahab Mohammad 3 Abdelbaki Benamor 4 Daniel Johnson 0000-0001-6921-0389 5 Nidal Hilal 6 0030211-28092016164016.pdf DES_Manuscript_ZnOGO_cyt-revised.pdf 2016-09-28T16:40:16.7370000 Output 1291734 application/pdf Accepted Manuscript true 2017-10-11T00:00:00.0000000 false
title Development of polysulfone-nanohybrid membranes using ZnO-GO composite for enhanced antifouling and antibacterial control
spellingShingle Development of polysulfone-nanohybrid membranes using ZnO-GO composite for enhanced antifouling and antibacterial control
Daniel Johnson
Nidal Hilal
title_short Development of polysulfone-nanohybrid membranes using ZnO-GO composite for enhanced antifouling and antibacterial control
title_full Development of polysulfone-nanohybrid membranes using ZnO-GO composite for enhanced antifouling and antibacterial control
title_fullStr Development of polysulfone-nanohybrid membranes using ZnO-GO composite for enhanced antifouling and antibacterial control
title_full_unstemmed Development of polysulfone-nanohybrid membranes using ZnO-GO composite for enhanced antifouling and antibacterial control
title_sort Development of polysulfone-nanohybrid membranes using ZnO-GO composite for enhanced antifouling and antibacterial control
author_id_str_mv 4bdcc306062428d2715b0dd308cc092f
3acba771241d878c8e35ff464aec0342
author_id_fullname_str_mv 4bdcc306062428d2715b0dd308cc092f_***_Daniel Johnson
3acba771241d878c8e35ff464aec0342_***_Nidal Hilal
author Daniel Johnson
Nidal Hilal
author2 Ying Tao Chung
Ebrahim Mahmoudi
Abdul Wahab Mohammad
Abdelbaki Benamor
Daniel Johnson
Nidal Hilal
format Journal article
container_title Desalination
container_volume 402
container_start_page 123
publishDate 2017
institution Swansea University
issn 0011-9164
doi_str_mv 10.1016/j.desal.2016.09.030
college_str Faculty of Science and Engineering
hierarchytype
hierarchy_top_id facultyofscienceandengineering
hierarchy_top_title Faculty of Science and Engineering
hierarchy_parent_id facultyofscienceandengineering
hierarchy_parent_title Faculty of Science and Engineering
department_str School of Engineering and Applied Sciences - Uncategorised{{{_:::_}}}Faculty of Science and Engineering{{{_:::_}}}School of Engineering and Applied Sciences - Uncategorised
document_store_str 1
active_str 0
description Zinc oxide nanoparticles were well-known for the enhanced antifouling and antibacterial properties which could be beneficial for membrane processes in desalination. The functionalization of ZnO onto graphene oxide nanoplates was targeted for better distribution. Both ZnO and ZnO-GO NPs were synthesized using sol-gel method. The nanoparticles characteristics were checked with XRD, TEM, and FESEM. The nanohybrid membranes were fabricated via wet phase inversion technique and embedded with various percentage of ZnO (1, 2, 3 wt%) and ZnO-GO (0.1, 0.3, 0.6 wt%) nanoparticles. All the membranes with nanoparticles incorporation exhibited improved membrane properties in comparison with the pristine PSF membrane. The best membrane performance was shown in membrane with 2 wt% of ZnO and 0.6 wt% of ZnO-GO. These two membranes presented significantly improved performance such as enhanced hydrophilicity, high permeability and porosity, improved humic acid rejection rate as well as good antifouling and antibacterial control. To an extent, the excellent antimicrobial ability of these nanohybrid membranes appeared as appropriate candidate to contribute or overcome bio-fouling issues in applications such as brackish water or seawater desalination. Hence, ZnO and ZnO-GO NPs were superb nanomaterials in the fabrication of PSF-nanohybrid membranes. The use of GO nanoplates allowed reduction of ZnO composition by up to 5 times while showing similar performances.
published_date 2017-01-16T03:36:50Z
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score 11.013619

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