One-step deposition by slot-die coating of mixed lead halide perovskite for photovoltaic applications

Cotella, Giovanni; Baker, Jenny; Worsley, David; Rossi, Francesca De; Pleydell-Pearce, Cameron; Carnie, Matt; Watson, Trystan

doi:10.1016/j.solmat.2016.09.013

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One-step deposition by slot-die coating of mixed lead halide perovskite for photovoltaic applications

Giovanni Cotella, Jenny Baker

, David Worsley

, Francesca De Rossi

, Cameron Pleydell-Pearce, Matt Carnie

, Trystan Watson

Solar Energy Materials and Solar Cells, Volume: 159, Pages: 362 - 369

Swansea University Authors: Jenny Baker , David Worsley , Francesca De Rossi , Cameron Pleydell-Pearce, Matt Carnie , Trystan Watson

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DOI (Published version): 10.1016/j.solmat.2016.09.013

Abstract

Recent advances in the performance and stability of lead halide perovskite solar cells announce a promising future for this technology. As the understanding of lab scale device fabrication progresses technology developments in the area of up-scaling are required to demonstrate their viability on an...

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Published in:	Solar Energy Materials and Solar Cells
ISSN:	0927-0248
Published:	2017
Online Access:	Check full text
URI:	https://cronfa.swan.ac.uk/Record/cronfa29891
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first_indexed	2016-09-12T13:02:29Z
last_indexed	2021-01-15T03:47:50Z
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spelling	2021-01-14T13:11:14.9717453 v2 29891 2016-09-12 One-step deposition by slot-die coating of mixed lead halide perovskite for photovoltaic applications 6913b56f36f0c8cd34d8c9040d2df460 0000-0003-3530-1957 Jenny Baker Jenny Baker true false c426b1c1b0123d7057c1b969083cea69 0000-0002-9956-6228 David Worsley David Worsley true false 04b56f7760ea2de5fd65985ff510d625 0000-0002-6591-5928 Francesca De Rossi Francesca De Rossi true false 564c480cb2abe761533a139c7dbaaca1 Cameron Pleydell-Pearce Cameron Pleydell-Pearce true false 73b367694366a646b90bb15db32bb8c0 0000-0002-4232-1967 Matt Carnie Matt Carnie true false a210327b52472cfe8df9b8108d661457 0000-0002-8015-1436 Trystan Watson Trystan Watson true false 2016-09-12 MECH Recent advances in the performance and stability of lead halide perovskite solar cells announce a promising future for this technology. As the understanding of lab scale device fabrication progresses technology developments in the area of up-scaling are required to demonstrate their viability on an industrial and pre-commercial scale. These developments include replacing slow spin coated deposition techniques with continuous roll to roll compatible slot-die methods. In this work we demonstrate the suitability of a one-step slot-die coating method for the deposition of lead halide perovskite layers, in particular for infiltration into a mesoporous titania scaffold. Appropriate crystallisation dynamics of the perovskite are achieved by careful control of the substrate temperature in combination with a post-processed rapid air knife application. We show that devices fully processed in air using this method deliver a photovoltaic conversion efficiency up to 9.2%, this is comparable to those manufactured using a spin coating process. Journal Article Solar Energy Materials and Solar Cells 159 362 369 0927-0248 Perovskite; Slot-die; Printing; One-step; Photovoltaic 1 1 2017 2017-01-01 10.1016/j.solmat.2016.09.013 COLLEGE NANME Mechanical Engineering COLLEGE CODE MECH Swansea University 2021-01-14T13:11:14.9717453 2016-09-12T08:51:12.1069471 Faculty of Science and Engineering School of Engineering and Applied Sciences - Materials Science and Engineering Giovanni Cotella 1 Jenny Baker 0000-0003-3530-1957 2 David Worsley 0000-0002-9956-6228 3 Francesca De Rossi 0000-0002-6591-5928 4 Cameron Pleydell-Pearce 5 Matt Carnie 0000-0002-4232-1967 6 Trystan Watson 0000-0002-8015-1436 7 0029891-12092016085143.pdf cotella2016.pdf 2016-09-12T08:51:43.7770000 Output 12020820 application/pdf Accepted Manuscript true 2017-09-30T00:00:00.0000000 Released under the terms of a Creative Commons Attribution Non-Commercial No Derivatives License (CC-BY-NC-ND). true eng
title	One-step deposition by slot-die coating of mixed lead halide perovskite for photovoltaic applications
spellingShingle	One-step deposition by slot-die coating of mixed lead halide perovskite for photovoltaic applications Jenny Baker David Worsley Francesca De Rossi Cameron Pleydell-Pearce Matt Carnie Trystan Watson
title_short	One-step deposition by slot-die coating of mixed lead halide perovskite for photovoltaic applications
title_full	One-step deposition by slot-die coating of mixed lead halide perovskite for photovoltaic applications
title_fullStr	One-step deposition by slot-die coating of mixed lead halide perovskite for photovoltaic applications
title_full_unstemmed	One-step deposition by slot-die coating of mixed lead halide perovskite for photovoltaic applications
title_sort	One-step deposition by slot-die coating of mixed lead halide perovskite for photovoltaic applications
author_id_str_mv	6913b56f36f0c8cd34d8c9040d2df460 c426b1c1b0123d7057c1b969083cea69 04b56f7760ea2de5fd65985ff510d625 564c480cb2abe761533a139c7dbaaca1 73b367694366a646b90bb15db32bb8c0 a210327b52472cfe8df9b8108d661457
author_id_fullname_str_mv	6913b56f36f0c8cd34d8c9040d2df460_*_Jenny Baker c426b1c1b0123d7057c1b969083cea69__David Worsley 04b56f7760ea2de5fd65985ff510d625__Francesca De Rossi 564c480cb2abe761533a139c7dbaaca1__Cameron Pleydell-Pearce 73b367694366a646b90bb15db32bb8c0__Matt Carnie a210327b52472cfe8df9b8108d661457_*_Trystan Watson
author	Jenny Baker David Worsley Francesca De Rossi Cameron Pleydell-Pearce Matt Carnie Trystan Watson
author2	Giovanni Cotella Jenny Baker David Worsley Francesca De Rossi Cameron Pleydell-Pearce Matt Carnie Trystan Watson
format	Journal article
container_title	Solar Energy Materials and Solar Cells
container_volume	159
container_start_page	362
publishDate	2017
institution	Swansea University
issn	0927-0248
doi_str_mv	10.1016/j.solmat.2016.09.013
college_str	Faculty of Science and Engineering
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hierarchy_parent_title	Faculty of Science and Engineering
department_str	School of Engineering and Applied Sciences - Materials Science and Engineering{{{_:::_}}}Faculty of Science and Engineering{{{_:::_}}}School of Engineering and Applied Sciences - Materials Science and Engineering
document_store_str	1
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description	Recent advances in the performance and stability of lead halide perovskite solar cells announce a promising future for this technology. As the understanding of lab scale device fabrication progresses technology developments in the area of up-scaling are required to demonstrate their viability on an industrial and pre-commercial scale. These developments include replacing slow spin coated deposition techniques with continuous roll to roll compatible slot-die methods. In this work we demonstrate the suitability of a one-step slot-die coating method for the deposition of lead halide perovskite layers, in particular for infiltration into a mesoporous titania scaffold. Appropriate crystallisation dynamics of the perovskite are achieved by careful control of the substrate temperature in combination with a post-processed rapid air knife application. We show that devices fully processed in air using this method deliver a photovoltaic conversion efficiency up to 9.2%, this is comparable to those manufactured using a spin coating process.
published_date	2017-01-01T03:36:27Z
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score	11.036531

One-step deposition by slot-die coating of mixed lead halide perovskite for photovoltaic applications

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