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Enhancing Membrane Materials for Efficient Li Recycling and Recovery

Xingpeng Tian, Chunchun Ye, Liyuan Zhang Orcid Logo, Manoj K. Sugumar, Yan Zhao, Neil B. McKeown, Serena Margadonna Orcid Logo, Rui Tan Orcid Logo

Advanced Materials, Start page: 2402335

Swansea University Authors: Serena Margadonna Orcid Logo, Rui Tan Orcid Logo

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DOI (Published version): 10.1002/adma.202402335

Abstract

Rapid uptake of lithium-centric technology, e.g., electric vehicles and large-scale energy storage, is increasing the demand for efficient technologies for lithium extraction from aqueous sources. Among various lithium-extraction technologies, membrane processes hold great promise due to energy effi...

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Published in: Advanced Materials
ISSN: 0935-9648 1521-4095
Published: Wiley 2024
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URI: https://cronfa.swan.ac.uk/Record/cronfa67974
first_indexed 2024-10-14T07:39:41Z
last_indexed 2025-01-09T20:32:16Z
id cronfa67974
recordtype SURis
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spelling 2024-12-16T15:29:21.1222341 v2 67974 2024-10-14 Enhancing Membrane Materials for Efficient Li Recycling and Recovery e31904a10b1b1240b98ab52d9977dfbe 0000-0002-6996-6562 Serena Margadonna Serena Margadonna true false 774c33a0a76a9152ca86a156b5ae26ff 0009-0001-9278-7327 Rui Tan Rui Tan true false 2024-10-14 EAAS Rapid uptake of lithium-centric technology, e.g., electric vehicles and large-scale energy storage, is increasing the demand for efficient technologies for lithium extraction from aqueous sources. Among various lithium-extraction technologies, membrane processes hold great promise due to energy efficiency and flexible operation in a continuous process with potential commercial viability. However, membrane separators face challenges such as the extraction efficiency due to the limited selectivity toward lithium relative to other species. Low selectivity can be ascribed to the uncontrollable selective channels and inefficient exclusion functions. However, recent selectivity enhancements for other membrane applications, such as in gas separation and energy storage, suggest that this may also be possible for lithium extraction. This review article focuses on the innovations in the membrane chemistries based on rational design following separation principles and unveiling the theories behind enhanced selectivity. Furthermore, recent progress in membrane-based lithium extraction technologies is summarized with the emphasis on inorganic, organic, and composite materials. The challenges and opportunities for developing the next generation of selective membranes for lithium recovery are also pointed out. Journal Article Advanced Materials 0 2402335 Wiley 0935-9648 1521-4095 Lithium extraction and recovery, lithium transport mechanisms, membranes, separation 15 12 2024 2024-12-15 10.1002/adma.202402335 Review COLLEGE NANME Engineering and Applied Sciences School COLLEGE CODE EAAS Swansea University SU Library paid the OA fee (TA Institutional Deal) X.T. and C.Y. contributed equally to this work. R.T. acknowledges the support from Royal Academy of Enginnering, Royal Society Chemistry (RSC), RSC researcher collaboration grant (C23-8220221815) and Royce Industrial Collaboration Grant (RICP-R4-100029). 2024-12-16T15:29:21.1222341 2024-10-14T08:20:32.5769989 Faculty of Science and Engineering School of Engineering and Applied Sciences - Chemical Engineering Xingpeng Tian 1 Chunchun Ye 2 Liyuan Zhang https://orcid.org/0000-0002-7585-5607 3 Manoj K. Sugumar 4 Yan Zhao 5 Neil B. McKeown 6 Serena Margadonna 0000-0002-6996-6562 7 Rui Tan 0009-0001-9278-7327 8
title Enhancing Membrane Materials for Efficient Li Recycling and Recovery
spellingShingle Enhancing Membrane Materials for Efficient Li Recycling and Recovery
Serena Margadonna
Rui Tan
title_short Enhancing Membrane Materials for Efficient Li Recycling and Recovery
title_full Enhancing Membrane Materials for Efficient Li Recycling and Recovery
title_fullStr Enhancing Membrane Materials for Efficient Li Recycling and Recovery
title_full_unstemmed Enhancing Membrane Materials for Efficient Li Recycling and Recovery
title_sort Enhancing Membrane Materials for Efficient Li Recycling and Recovery
author_id_str_mv e31904a10b1b1240b98ab52d9977dfbe
774c33a0a76a9152ca86a156b5ae26ff
author_id_fullname_str_mv e31904a10b1b1240b98ab52d9977dfbe_***_Serena Margadonna
774c33a0a76a9152ca86a156b5ae26ff_***_Rui Tan
author Serena Margadonna
Rui Tan
author2 Xingpeng Tian
Chunchun Ye
Liyuan Zhang
Manoj K. Sugumar
Yan Zhao
Neil B. McKeown
Serena Margadonna
Rui Tan
format Journal article
container_title Advanced Materials
container_volume 0
container_start_page 2402335
publishDate 2024
institution Swansea University
issn 0935-9648
1521-4095
doi_str_mv 10.1002/adma.202402335
publisher Wiley
college_str Faculty of Science and Engineering
hierarchytype
hierarchy_top_id facultyofscienceandengineering
hierarchy_top_title Faculty of Science and Engineering
hierarchy_parent_id facultyofscienceandengineering
hierarchy_parent_title Faculty of Science and Engineering
department_str School of Engineering and Applied Sciences - Chemical Engineering{{{_:::_}}}Faculty of Science and Engineering{{{_:::_}}}School of Engineering and Applied Sciences - Chemical Engineering
document_store_str 0
active_str 0
description Rapid uptake of lithium-centric technology, e.g., electric vehicles and large-scale energy storage, is increasing the demand for efficient technologies for lithium extraction from aqueous sources. Among various lithium-extraction technologies, membrane processes hold great promise due to energy efficiency and flexible operation in a continuous process with potential commercial viability. However, membrane separators face challenges such as the extraction efficiency due to the limited selectivity toward lithium relative to other species. Low selectivity can be ascribed to the uncontrollable selective channels and inefficient exclusion functions. However, recent selectivity enhancements for other membrane applications, such as in gas separation and energy storage, suggest that this may also be possible for lithium extraction. This review article focuses on the innovations in the membrane chemistries based on rational design following separation principles and unveiling the theories behind enhanced selectivity. Furthermore, recent progress in membrane-based lithium extraction technologies is summarized with the emphasis on inorganic, organic, and composite materials. The challenges and opportunities for developing the next generation of selective membranes for lithium recovery are also pointed out.
published_date 2024-12-15T20:35:13Z
_version_ 1821348529124147200
score 11.04748

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