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Material Engineering Strategies for Efficient Hydrogen Evolution Reaction Catalysts

Yue Luo, Yulong Zhang, Jiayi Zhu, Xingpeng Tian, Gang Liu, Zhiming Feng, Liwen Pan, Xinhua Liu, Ning Han, Rui Tan Orcid Logo

Small Methods

Swansea University Author: Rui Tan Orcid Logo

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DOI (Published version): 10.1002/smtd.202400158

Abstract

Water electrolysis, a key enabler of hydrogen energy production, presents significant potential as a strategy for achieving net-zero emissions. However, the widespread deployment of water electrolysis is currently limited by the high-cost and scarce noble metal electrocatalysts in hydrogen evolution...

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Published in: Small Methods
ISSN: 2366-9608 2366-9608
Published: Wiley 2024
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URI: https://cronfa.swan.ac.uk/Record/cronfa67791
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Given this challenge, design and synthesis of cost-effective and high-performance alternative catalysts have become a research focus, which necessitates insightful understandings of HER fundamentals and material engineering strategies. Distinct from typical reviews that concentrate only on the summary of recent catalyst materials, this review article shifts focus to material engineering strategies for developing efficient HER catalysts. In-depth analysis of key material design approaches for HER catalysts, such as doping, vacancy defect creation, phase engineering, and metal-support engineering, are illustrated along with typical research cases. A special emphasis is placed on designing noble metal-free catalysts with a brief discussion on recent advancements in electrocatalytic water-splitting technology. 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spelling v2 67791 2024-09-25 Material Engineering Strategies for Efficient Hydrogen Evolution Reaction Catalysts 774c33a0a76a9152ca86a156b5ae26ff 0009-0001-9278-7327 Rui Tan Rui Tan true false 2024-09-25 EAAS Water electrolysis, a key enabler of hydrogen energy production, presents significant potential as a strategy for achieving net-zero emissions. However, the widespread deployment of water electrolysis is currently limited by the high-cost and scarce noble metal electrocatalysts in hydrogen evolution reaction (HER). Given this challenge, design and synthesis of cost-effective and high-performance alternative catalysts have become a research focus, which necessitates insightful understandings of HER fundamentals and material engineering strategies. Distinct from typical reviews that concentrate only on the summary of recent catalyst materials, this review article shifts focus to material engineering strategies for developing efficient HER catalysts. In-depth analysis of key material design approaches for HER catalysts, such as doping, vacancy defect creation, phase engineering, and metal-support engineering, are illustrated along with typical research cases. A special emphasis is placed on designing noble metal-free catalysts with a brief discussion on recent advancements in electrocatalytic water-splitting technology. The article also delves into important descriptors, reliable evaluation parameters and characterization techniques, aiming to link the fundamental mechanisms of HER with its catalytic performance. In conclusion, it explores future trends in HER catalysts by integrating theoretical, experimental and industrial perspectives, while acknowledging the challenges that remain. Journal Article Small Methods 0 Wiley 2366-9608 2366-9608 catalytic materials; design principles; hydrogen evolution reaction; material engineering strategies; noble metal-free catalysts 15 5 2024 2024-05-15 10.1002/smtd.202400158 COLLEGE NANME Engineering and Applied Sciences School COLLEGE CODE EAAS Swansea University Another institution paid the OA fee Warwick Manufacturing Group at the University of Warwick Key research and development plan project of Guangxi. Grant Number: GuiKeAB22080015 RSC Researcher Collaborations Grant. Grant Number: C23-8220221815 Specific Research Project of Guangxi for Research Bases and Talents. Grant Number: GuiKeAD21238010 2024-10-18T13:06:56.1120655 2024-09-25T21:17:44.5408062 Faculty of Science and Engineering School of Engineering and Applied Sciences - Chemical Engineering Yue Luo 1 Yulong Zhang 2 Jiayi Zhu 3 Xingpeng Tian 4 Gang Liu 5 Zhiming Feng 6 Liwen Pan 7 Xinhua Liu 8 Ning Han 9 Rui Tan 0009-0001-9278-7327 10 67791__32641__b00c970713a14f58bce0a2f90ed38e50.pdf 67791.VoR.pdf 2024-10-18T12:50:00.7375294 Output 1174236 application/pdf Version of Record true © 2024 The Authors. This is an open access article under the terms of the Creative Commons Attribution License. true eng http://creativecommons.org/licenses/by/4.0/
title Material Engineering Strategies for Efficient Hydrogen Evolution Reaction Catalysts
spellingShingle Material Engineering Strategies for Efficient Hydrogen Evolution Reaction Catalysts
Rui Tan
title_short Material Engineering Strategies for Efficient Hydrogen Evolution Reaction Catalysts
title_full Material Engineering Strategies for Efficient Hydrogen Evolution Reaction Catalysts
title_fullStr Material Engineering Strategies for Efficient Hydrogen Evolution Reaction Catalysts
title_full_unstemmed Material Engineering Strategies for Efficient Hydrogen Evolution Reaction Catalysts
title_sort Material Engineering Strategies for Efficient Hydrogen Evolution Reaction Catalysts
author_id_str_mv 774c33a0a76a9152ca86a156b5ae26ff
author_id_fullname_str_mv 774c33a0a76a9152ca86a156b5ae26ff_***_Rui Tan
author Rui Tan
author2 Yue Luo
Yulong Zhang
Jiayi Zhu
Xingpeng Tian
Gang Liu
Zhiming Feng
Liwen Pan
Xinhua Liu
Ning Han
Rui Tan
format Journal article
container_title Small Methods
container_volume 0
publishDate 2024
institution Swansea University
issn 2366-9608
2366-9608
doi_str_mv 10.1002/smtd.202400158
publisher Wiley
college_str Faculty of Science and Engineering
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hierarchy_top_id facultyofscienceandengineering
hierarchy_top_title Faculty of Science and Engineering
hierarchy_parent_id facultyofscienceandengineering
hierarchy_parent_title Faculty of Science and Engineering
department_str School of Engineering and Applied Sciences - Chemical Engineering{{{_:::_}}}Faculty of Science and Engineering{{{_:::_}}}School of Engineering and Applied Sciences - Chemical Engineering
document_store_str 1
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description Water electrolysis, a key enabler of hydrogen energy production, presents significant potential as a strategy for achieving net-zero emissions. However, the widespread deployment of water electrolysis is currently limited by the high-cost and scarce noble metal electrocatalysts in hydrogen evolution reaction (HER). Given this challenge, design and synthesis of cost-effective and high-performance alternative catalysts have become a research focus, which necessitates insightful understandings of HER fundamentals and material engineering strategies. Distinct from typical reviews that concentrate only on the summary of recent catalyst materials, this review article shifts focus to material engineering strategies for developing efficient HER catalysts. In-depth analysis of key material design approaches for HER catalysts, such as doping, vacancy defect creation, phase engineering, and metal-support engineering, are illustrated along with typical research cases. A special emphasis is placed on designing noble metal-free catalysts with a brief discussion on recent advancements in electrocatalytic water-splitting technology. The article also delves into important descriptors, reliable evaluation parameters and characterization techniques, aiming to link the fundamental mechanisms of HER with its catalytic performance. In conclusion, it explores future trends in HER catalysts by integrating theoretical, experimental and industrial perspectives, while acknowledging the challenges that remain.
published_date 2024-05-15T13:06:54Z
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