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Fast-Response Photodetector Based on Hybrid Bi2Te3/PbS Colloidal Quantum Dots

Lijing Yu, Pin Tian, Libin Tang, Qun Hao, Vincent Teng Orcid Logo, Hefu Zhong, Biao Yue, Haipeng Wang, Shunying Yan

Nanomaterials, Volume: 12, Issue: 18, Start page: 3212

Swansea University Author: Vincent Teng Orcid Logo

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DOI (Published version): 10.3390/nano12183212

Abstract

Colloidal quantum dots (CQDs) as photodetector materials have attracted much attention in recent years due to their tunable energy bands, low cost, and solution processability. However, their intrinsically low carrier mobility and three-dimensional (3D) confinement of charges are unsuitable for use...

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Published in: Nanomaterials
ISSN: 2079-4991
Published: MDPI AG 2022
Online Access: Check full text

URI: https://cronfa.swan.ac.uk/Record/cronfa61286
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Abstract: Colloidal quantum dots (CQDs) as photodetector materials have attracted much attention in recent years due to their tunable energy bands, low cost, and solution processability. However, their intrinsically low carrier mobility and three-dimensional (3D) confinement of charges are unsuitable for use in fast-response and highly sensitive photodetectors, hence greatly restricting their application in many fields. Currently, 3D topological insulators, such as bismuth telluride (Bi2Te3), have been employed in high-speed broadband photodetectors due to their narrow bulk bandgap, high carrier mobility, and strong light absorption. In this work, the advantages of topological insulators and CQDs were realized by developing a hybrid Bi2Te3/PbS CQDs photodetector that exhibited a maximum responsivity and detectivity of 18 A/W and 2.1 × 1011 Jones, respectively, with a rise time of 128 μs at 660 nm light illumination. The results indicate that such a photodetector has potential application in the field of fast-response and large-scale integrated optoelectronic devices.
Keywords: PbS; colloidal quantum dots; Bi2Te3; photodetector; hybrid
College: Faculty of Science and Engineering
Funders: This work was supported by the Yunnan Province Innovation Team Project (2018HC020) and National Key Research and Development Program of China (2019YFB2203404).
Issue: 18
Start Page: 3212