Scribing Method for Carbon Perovskite Solar Modules

Meroni, Simone; Hooper, Katherine; Dunlop, Tom O.; Baker, Jenny; Worsley, David; Charbonneau, Cecile; Watson, Trystan; Anne, Katherine Elizabeth; Dunlop, Tom

doi:10.3390/en13071589

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Scribing Method for Carbon Perovskite Solar Modules

Simone Meroni

, Katherine Hooper, Tom O. Dunlop

, Jenny Baker

, David Worsley

, Cecile Charbonneau

, Trystan Watson

, Katherine Elizabeth Anne Hooper

, Tom Dunlop

Energies, Volume: 13, Issue: 7, Start page: 1589

Swansea University Authors: Simone Meroni , Katherine Hooper, Tom O. Dunlop , Jenny Baker , David Worsley , Cecile Charbonneau , Trystan Watson , Katherine Elizabeth Anne Hooper , Tom Dunlop

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DOI (Published version): 10.3390/en13071589

Abstract

The fully printable carbon triple-mesoscopic perovskite solar cell (C-PSC) has already demonstrated good efficiency and long-term stability, opening the possibility of lab-to-fab transition. Modules based on C-PSC architecture have been reported and, at present, are achieved through the accurate reg...

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Published in:	Energies
ISSN:	1996-1073
Published:	MDPI AG 2020
Online Access:	Check full text
URI:	https://cronfa.swan.ac.uk/Record/cronfa53872
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Modules based on C-PSC architecture have been reported and, at present, are achieved through the accurate registration of each of the patterned layers using screen-printing. Modules based on this approach were reported with geometric fill factor (g-FF) as high as 70%. Another approach to create the interconnects, the so-called scribing method, was reported to achieve more than 90% g-FF for architectures based on evaporated metal contacts, i.e., without a carbon counter electrode. Here, for the first time, we adopt the scribing method to selectively remove materials within a C-PSC. This approach allowed a deep and selective scribe to open an aperture from the transparent electrode through all the layers, including the blocking layer, enabling a direct contact between the electrodes in the interconnects. In this work, a systematic study of the interconnection area between cells is discussed, showing the key role of the FTO/carbon contact. Furthermore, a module on 10 × 10 cm2 substrate with the optimised design showing efficiency over 10% is also demonstrated.</abstract><type>Journal Article</type><journal>Energies</journal><volume>13</volume><journalNumber>7</journalNumber><paginationStart>1589</paginationStart><publisher>MDPI AG</publisher><issnElectronic>1996-1073</issnElectronic><keywords>perovskite; solar cells; carbon; screen-printing; up-scaling; module; scribing</keywords><publishedDay>1</publishedDay><publishedMonth>4</publishedMonth><publishedYear>2020</publishedYear><publishedDate>2020-04-01</publishedDate><doi>10.3390/en13071589</doi><url/><notes/><college>COLLEGE NANME</college><department>Materials Science and Engineering</department><CollegeCode>COLLEGE CODE</CollegeCode><DepartmentCode>MTLS</DepartmentCode><institution>Swansea University</institution><apcterm/><lastEdited>2020-07-06T17:08:39.5697851</lastEdited><Created>2020-03-27T09:17:18.8146131</Created><authors><author><firstname>Simone</firstname><surname>Meroni</surname><orcid>0000-0002-6901-772X</orcid><order>1</order></author><author><firstname>Katherine</firstname><surname>Hooper</surname><order>2</order></author><author><firstname>Tom O.</firstname><surname>Dunlop</surname><orcid>0000-0002-5851-8713</orcid><order>3</order></author><author><firstname>Jenny</firstname><surname>Baker</surname><orcid>0000-0003-3530-1957</orcid><order>4</order></author><author><firstname>David</firstname><surname>Worsley</surname><orcid>0000-0002-9956-6228</orcid><order>5</order></author><author><firstname>Cecile</firstname><surname>Charbonneau</surname><orcid>0000-0001-9887-2007</orcid><order>6</order></author><author><firstname>Trystan</firstname><surname>Watson</surname><orcid>0000-0002-8015-1436</orcid><order>7</order></author><author><firstname>Katherine Elizabeth Anne</firstname><surname>Hooper</surname><orcid>NULL</orcid><order>8</order></author><author><firstname>Tom</firstname><surname>Dunlop</surname><orcid>0000-0002-5851-8713</orcid><order>9</order></author></authors><documents><document><filename>53872__16991__a9c21a1a6ded4336825a2e903268f58d.pdf</filename><originalFilename>53872.pdf</originalFilename><uploaded>2020-04-02T10:41:36.8236788</uploaded><type>Output</type><contentLength>4462202</contentLength><contentType>application/pdf</contentType><version>Version of Record</version><cronfaStatus>true</cronfaStatus><documentNotes>Released under the terms of a Creative Commons Attribution License (CC-BY).</documentNotes><copyrightCorrect>true</copyrightCorrect><language>eng</language><licence>http://creativecommons.org/licenses/by/4.0/</licence></document></documents><OutputDurs/></rfc1807>
spelling	2020-07-06T17:08:39.5697851 v2 53872 2020-03-27 Scribing Method for Carbon Perovskite Solar Modules 78a4cf80ab2fe6cca80716b5d357d8dd 0000-0002-6901-772X Simone Meroni Simone Meroni true false 3607f6787dc810c0ed1fdc49ea2b5e63 Katherine Hooper Katherine Hooper true false 2c5194f421c9fe645b6115c20f5cf9ad 0000-0002-5851-8713 Tom O. Dunlop Tom O. Dunlop true true 6913b56f36f0c8cd34d8c9040d2df460 0000-0003-3530-1957 Jenny Baker Jenny Baker true false c426b1c1b0123d7057c1b969083cea69 0000-0002-9956-6228 David Worsley David Worsley true false 4dc059714847cb22ed922ab058950560 0000-0001-9887-2007 Cecile Charbonneau Cecile Charbonneau true false a210327b52472cfe8df9b8108d661457 0000-0002-8015-1436 Trystan Watson Trystan Watson true false 05bbb9d0476050619f9a458278aeb62a NULL Katherine Elizabeth Anne Hooper Katherine Elizabeth Anne Hooper true true 809395460ab1e6b53a906b136d919c41 0000-0002-5851-8713 Tom Dunlop Tom Dunlop true false 2020-03-27 MTLS The fully printable carbon triple-mesoscopic perovskite solar cell (C-PSC) has already demonstrated good efficiency and long-term stability, opening the possibility of lab-to-fab transition. Modules based on C-PSC architecture have been reported and, at present, are achieved through the accurate registration of each of the patterned layers using screen-printing. Modules based on this approach were reported with geometric fill factor (g-FF) as high as 70%. Another approach to create the interconnects, the so-called scribing method, was reported to achieve more than 90% g-FF for architectures based on evaporated metal contacts, i.e., without a carbon counter electrode. Here, for the first time, we adopt the scribing method to selectively remove materials within a C-PSC. This approach allowed a deep and selective scribe to open an aperture from the transparent electrode through all the layers, including the blocking layer, enabling a direct contact between the electrodes in the interconnects. In this work, a systematic study of the interconnection area between cells is discussed, showing the key role of the FTO/carbon contact. Furthermore, a module on 10 × 10 cm2 substrate with the optimised design showing efficiency over 10% is also demonstrated. Journal Article Energies 13 7 1589 MDPI AG 1996-1073 perovskite; solar cells; carbon; screen-printing; up-scaling; module; scribing 1 4 2020 2020-04-01 10.3390/en13071589 COLLEGE NANME Materials Science and Engineering COLLEGE CODE MTLS Swansea University 2020-07-06T17:08:39.5697851 2020-03-27T09:17:18.8146131 Simone Meroni 0000-0002-6901-772X 1 Katherine Hooper 2 Tom O. Dunlop 0000-0002-5851-8713 3 Jenny Baker 0000-0003-3530-1957 4 David Worsley 0000-0002-9956-6228 5 Cecile Charbonneau 0000-0001-9887-2007 6 Trystan Watson 0000-0002-8015-1436 7 Katherine Elizabeth Anne Hooper NULL 8 Tom Dunlop 0000-0002-5851-8713 9 53872__16991__a9c21a1a6ded4336825a2e903268f58d.pdf 53872.pdf 2020-04-02T10:41:36.8236788 Output 4462202 application/pdf Version of Record true Released under the terms of a Creative Commons Attribution License (CC-BY). true eng http://creativecommons.org/licenses/by/4.0/
title	Scribing Method for Carbon Perovskite Solar Modules
spellingShingle	Scribing Method for Carbon Perovskite Solar Modules Simone Meroni Katherine Hooper Tom O. Dunlop Jenny Baker David Worsley Cecile Charbonneau Trystan Watson Katherine Elizabeth Anne Hooper Tom Dunlop
title_short	Scribing Method for Carbon Perovskite Solar Modules
title_full	Scribing Method for Carbon Perovskite Solar Modules
title_fullStr	Scribing Method for Carbon Perovskite Solar Modules
title_full_unstemmed	Scribing Method for Carbon Perovskite Solar Modules
title_sort	Scribing Method for Carbon Perovskite Solar Modules
author_id_str_mv	78a4cf80ab2fe6cca80716b5d357d8dd 3607f6787dc810c0ed1fdc49ea2b5e63 2c5194f421c9fe645b6115c20f5cf9ad 6913b56f36f0c8cd34d8c9040d2df460 c426b1c1b0123d7057c1b969083cea69 4dc059714847cb22ed922ab058950560 a210327b52472cfe8df9b8108d661457 05bbb9d0476050619f9a458278aeb62a 809395460ab1e6b53a906b136d919c41
author_id_fullname_str_mv	78a4cf80ab2fe6cca80716b5d357d8dd_*_Simone Meroni 3607f6787dc810c0ed1fdc49ea2b5e63__Katherine Hooper 2c5194f421c9fe645b6115c20f5cf9ad__Tom O. Dunlop 6913b56f36f0c8cd34d8c9040d2df460__Jenny Baker c426b1c1b0123d7057c1b969083cea69__David Worsley 4dc059714847cb22ed922ab058950560__Cecile Charbonneau a210327b52472cfe8df9b8108d661457__Trystan Watson 05bbb9d0476050619f9a458278aeb62a__Katherine Elizabeth Anne Hooper 809395460ab1e6b53a906b136d919c41_**_Tom Dunlop
author	Simone Meroni Katherine Hooper Tom O. Dunlop Jenny Baker David Worsley Cecile Charbonneau Trystan Watson Katherine Elizabeth Anne Hooper Tom Dunlop
author2	Simone Meroni Katherine Hooper Tom O. Dunlop Jenny Baker David Worsley Cecile Charbonneau Trystan Watson Katherine Elizabeth Anne Hooper Tom Dunlop
format	Journal article
container_title	Energies
container_volume	13
container_issue	7
container_start_page	1589
publishDate	2020
institution	Swansea University
issn	1996-1073
doi_str_mv	10.3390/en13071589
publisher	MDPI AG
document_store_str	1
active_str	0
description	The fully printable carbon triple-mesoscopic perovskite solar cell (C-PSC) has already demonstrated good efficiency and long-term stability, opening the possibility of lab-to-fab transition. Modules based on C-PSC architecture have been reported and, at present, are achieved through the accurate registration of each of the patterned layers using screen-printing. Modules based on this approach were reported with geometric fill factor (g-FF) as high as 70%. Another approach to create the interconnects, the so-called scribing method, was reported to achieve more than 90% g-FF for architectures based on evaporated metal contacts, i.e., without a carbon counter electrode. Here, for the first time, we adopt the scribing method to selectively remove materials within a C-PSC. This approach allowed a deep and selective scribe to open an aperture from the transparent electrode through all the layers, including the blocking layer, enabling a direct contact between the electrodes in the interconnects. In this work, a systematic study of the interconnection area between cells is discussed, showing the key role of the FTO/carbon contact. Furthermore, a module on 10 × 10 cm2 substrate with the optimised design showing efficiency over 10% is also demonstrated.
published_date	2020-04-01T04:07:04Z
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score	11.013371

Scribing Method for Carbon Perovskite Solar Modules

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