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Highly Ordered N‐Doped Carbon Dots Photosensitizer on Metal–Organic Framework‐Decorated ZnO Nanotubes for Improved Photoelectrochemical Water Splitting

Hyungkyu Han, Frantisek Karlicky, Sudhagar Pitchaimuthu Orcid Logo, Sun Hae Ra Shin, Aiping Chen

Small, Start page: 1902771

Swansea University Author: Sudhagar Pitchaimuthu Orcid Logo

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DOI (Published version): 10.1002/smll.201902771

Abstract

In spite of having several advantages such as low cost, high chemical stability, and environmentally safe and benign synthetic as well as operational procedures, the full potential of carbon dots (CDs) is yet to be explored as photosensitizers due to the challenges associated with the fabrication of...

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Published in: Small
ISSN: 1613-6810 1613-6829
Published: 2019
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URI: https://cronfa.swan.ac.uk/Record/cronfa51621
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first_indexed 2019-08-29T14:53:23Z
last_indexed 2021-09-25T03:11:38Z
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spelling 2021-09-24T15:28:54.3879912 v2 51621 2019-08-29 Highly Ordered N‐Doped Carbon Dots Photosensitizer on Metal–Organic Framework‐Decorated ZnO Nanotubes for Improved Photoelectrochemical Water Splitting 2fdbee02f4bfc5a1b174c8bd04afbd2b 0000-0001-9098-8806 Sudhagar Pitchaimuthu Sudhagar Pitchaimuthu true false 2019-08-29 EEN In spite of having several advantages such as low cost, high chemical stability, and environmentally safe and benign synthetic as well as operational procedures, the full potential of carbon dots (CDs) is yet to be explored as photosensitizers due to the challenges associated with the fabrication of well‐arrayed CDs with many other photocatalytic heterostructures. In the present study, a unique combination of metal–organic framework (MOF)‐decorated zinc oxide (ZnO) 1D nanostructures as host and CDs as guest species are explored on account of their potential application in photoelectrochemical (PEC) water splitting performance. The synthetic strategy to incorporate well‐defined nitrogen‐doped carbon dots (N‐CDs) arrays onto a zeolitic imidazolate framework‐8 (ZIF‐8) anchored on ZnO 1D nanostructures allows a facile unification of different components which subsequently plays a decisive role in improving the material's PEC water splitting performance. Simple extension of such strategies is expected to offer significant advantages for the preparation of CD‐based heterostructures for photo(electro)catalytics and other related applications. Journal Article Small 1902771 1613-6810 1613-6829 31 12 2019 2019-12-31 10.1002/smll.201902771 COLLEGE NANME Engineering COLLEGE CODE EEN Swansea University 2021-09-24T15:28:54.3879912 2019-08-29T10:18:56.8109167 Faculty of Science and Engineering School of Engineering and Applied Sciences - Uncategorised Hyungkyu Han 1 Frantisek Karlicky 2 Sudhagar Pitchaimuthu 0000-0001-9098-8806 3 Sun Hae Ra Shin 4 Aiping Chen 5
title Highly Ordered N‐Doped Carbon Dots Photosensitizer on Metal–Organic Framework‐Decorated ZnO Nanotubes for Improved Photoelectrochemical Water Splitting
spellingShingle Highly Ordered N‐Doped Carbon Dots Photosensitizer on Metal–Organic Framework‐Decorated ZnO Nanotubes for Improved Photoelectrochemical Water Splitting
Sudhagar Pitchaimuthu
title_short Highly Ordered N‐Doped Carbon Dots Photosensitizer on Metal–Organic Framework‐Decorated ZnO Nanotubes for Improved Photoelectrochemical Water Splitting
title_full Highly Ordered N‐Doped Carbon Dots Photosensitizer on Metal–Organic Framework‐Decorated ZnO Nanotubes for Improved Photoelectrochemical Water Splitting
title_fullStr Highly Ordered N‐Doped Carbon Dots Photosensitizer on Metal–Organic Framework‐Decorated ZnO Nanotubes for Improved Photoelectrochemical Water Splitting
title_full_unstemmed Highly Ordered N‐Doped Carbon Dots Photosensitizer on Metal–Organic Framework‐Decorated ZnO Nanotubes for Improved Photoelectrochemical Water Splitting
title_sort Highly Ordered N‐Doped Carbon Dots Photosensitizer on Metal–Organic Framework‐Decorated ZnO Nanotubes for Improved Photoelectrochemical Water Splitting
author_id_str_mv 2fdbee02f4bfc5a1b174c8bd04afbd2b
author_id_fullname_str_mv 2fdbee02f4bfc5a1b174c8bd04afbd2b_***_Sudhagar Pitchaimuthu
author Sudhagar Pitchaimuthu
author2 Hyungkyu Han
Frantisek Karlicky
Sudhagar Pitchaimuthu
Sun Hae Ra Shin
Aiping Chen
format Journal article
container_title Small
container_start_page 1902771
publishDate 2019
institution Swansea University
issn 1613-6810
1613-6829
doi_str_mv 10.1002/smll.201902771
college_str Faculty of Science and Engineering
hierarchytype
hierarchy_top_id facultyofscienceandengineering
hierarchy_top_title Faculty of Science and Engineering
hierarchy_parent_id facultyofscienceandengineering
hierarchy_parent_title Faculty of Science and Engineering
department_str School of Engineering and Applied Sciences - Uncategorised{{{_:::_}}}Faculty of Science and Engineering{{{_:::_}}}School of Engineering and Applied Sciences - Uncategorised
document_store_str 0
active_str 0
description In spite of having several advantages such as low cost, high chemical stability, and environmentally safe and benign synthetic as well as operational procedures, the full potential of carbon dots (CDs) is yet to be explored as photosensitizers due to the challenges associated with the fabrication of well‐arrayed CDs with many other photocatalytic heterostructures. In the present study, a unique combination of metal–organic framework (MOF)‐decorated zinc oxide (ZnO) 1D nanostructures as host and CDs as guest species are explored on account of their potential application in photoelectrochemical (PEC) water splitting performance. The synthetic strategy to incorporate well‐defined nitrogen‐doped carbon dots (N‐CDs) arrays onto a zeolitic imidazolate framework‐8 (ZIF‐8) anchored on ZnO 1D nanostructures allows a facile unification of different components which subsequently plays a decisive role in improving the material's PEC water splitting performance. Simple extension of such strategies is expected to offer significant advantages for the preparation of CD‐based heterostructures for photo(electro)catalytics and other related applications.
published_date 2019-12-31T04:03:35Z
_version_ 1763753292681183232
score 10.997456

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