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From fullerene acceptors to non-fullerene acceptors: prospects and challenges in the stability of organic solar cells

Emily M. Speller, Andrew J. Clarke, Joel Luke, Harrison Ka Hin Lee, Ning Li, Tao Wang, Him Cheng Wong, Ji-Seon Kim, Wing Chung Tsoi, Zhe Li

Journal of Materials Chemistry A

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DOI (Published version): 10.1039/C9TA05235F

Abstract

The recent emergence of non-fullerene small molecule acceptors has reinvigorated the field of organic solar cells, already resulting in significant breakthroughs in their power conversion efficiency and discovery of remarkable new science. The stability and degradation of this class of materials and...

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Published in: Journal of Materials Chemistry A
ISSN: 2050-7488 2050-7496
Published: 2019
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URI: https://cronfa.swan.ac.uk/Record/cronfa50960
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first_indexed 2019-06-28T14:55:51Z
last_indexed 2022-05-10T03:17:36Z
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spelling 2022-05-09T15:45:28.9013453 v2 50960 2019-06-28 From fullerene acceptors to non-fullerene acceptors: prospects and challenges in the stability of organic solar cells 2019-06-28 The recent emergence of non-fullerene small molecule acceptors has reinvigorated the field of organic solar cells, already resulting in significant breakthroughs in their power conversion efficiency and discovery of remarkable new science. The stability and degradation of this class of materials and devices, on the other hand, has to date received relatively less attention. Herein, we present a critical review into the fundamentally different degradation mechanisms of non-fullerene acceptors compared to fullerene acceptors, as well as the very different roles they play upon the charge carrier generation and recombination kinetics and the resulting solar cell stability. We highlight in particular the prospect of the emergence of non-fullerene acceptors in addressing several major degradation mechanisms related to the use of fullerene acceptors, in conjunction with a number of unique degradation mechanisms that only exist in non-fullerene acceptors, which would provide an important guideline for further developments toward achieving long-term stability of organic solar cells. Journal Article Journal of Materials Chemistry A 2050-7488 2050-7496 31 12 2019 2019-12-31 10.1039/C9TA05235F COLLEGE NANME COLLEGE CODE Swansea University 2022-05-09T15:45:28.9013453 2019-06-28T12:17:21.5212718 Faculty of Science and Engineering School of Engineering and Applied Sciences - Uncategorised Emily M. Speller 1 Andrew J. Clarke 2 Joel Luke 3 Harrison Ka Hin Lee 4 Ning Li 5 Tao Wang 6 Him Cheng Wong 7 Ji-Seon Kim 8 Wing Chung Tsoi 9 Zhe Li 10 0050960-28062019121947.pdf speller2019(2).pdf 2019-06-28T12:19:47.8770000 Output 878140 application/pdf Accepted Manuscript true 2020-06-26T00:00:00.0000000 false eng
title From fullerene acceptors to non-fullerene acceptors: prospects and challenges in the stability of organic solar cells
spellingShingle From fullerene acceptors to non-fullerene acceptors: prospects and challenges in the stability of organic solar cells
,
title_short From fullerene acceptors to non-fullerene acceptors: prospects and challenges in the stability of organic solar cells
title_full From fullerene acceptors to non-fullerene acceptors: prospects and challenges in the stability of organic solar cells
title_fullStr From fullerene acceptors to non-fullerene acceptors: prospects and challenges in the stability of organic solar cells
title_full_unstemmed From fullerene acceptors to non-fullerene acceptors: prospects and challenges in the stability of organic solar cells
title_sort From fullerene acceptors to non-fullerene acceptors: prospects and challenges in the stability of organic solar cells
author ,
author2 Emily M. Speller
Andrew J. Clarke
Joel Luke
Harrison Ka Hin Lee
Ning Li
Tao Wang
Him Cheng Wong
Ji-Seon Kim
Wing Chung Tsoi
Zhe Li
format Journal article
container_title Journal of Materials Chemistry A
publishDate 2019
institution Swansea University
issn 2050-7488
2050-7496
doi_str_mv 10.1039/C9TA05235F
college_str Faculty of Science and Engineering
hierarchytype
hierarchy_top_id facultyofscienceandengineering
hierarchy_top_title Faculty of Science and Engineering
hierarchy_parent_id facultyofscienceandengineering
hierarchy_parent_title Faculty of Science and Engineering
department_str School of Engineering and Applied Sciences - Uncategorised{{{_:::_}}}Faculty of Science and Engineering{{{_:::_}}}School of Engineering and Applied Sciences - Uncategorised
document_store_str 1
active_str 0
description The recent emergence of non-fullerene small molecule acceptors has reinvigorated the field of organic solar cells, already resulting in significant breakthroughs in their power conversion efficiency and discovery of remarkable new science. The stability and degradation of this class of materials and devices, on the other hand, has to date received relatively less attention. Herein, we present a critical review into the fundamentally different degradation mechanisms of non-fullerene acceptors compared to fullerene acceptors, as well as the very different roles they play upon the charge carrier generation and recombination kinetics and the resulting solar cell stability. We highlight in particular the prospect of the emergence of non-fullerene acceptors in addressing several major degradation mechanisms related to the use of fullerene acceptors, in conjunction with a number of unique degradation mechanisms that only exist in non-fullerene acceptors, which would provide an important guideline for further developments toward achieving long-term stability of organic solar cells.
published_date 2019-12-31T04:02:40Z
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score 11.013148

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